
Our unit aims to develop new magnetic materials with topological and high-performance magnetic functionalities. We focus on the exploration of novel intermetallic compounds and alloys using single-crystal growth and non-equilibrium methods, and elucidate their magnetic structures and topological properties through various experimental techniques, including magnetometry, electrical transport measurements, scanning probe microscopy, and neutron scattering.
Development of kagome lattice magnets hosting room-temperature skyrmions and large anomalous Hall effect
Magnetic materials with a kagome lattice have attracted considerable attention in recent years because their geometric structure gives rise to a variety of topological properties. However, materials that exhibit topological phenomena above room temperature have been limited so far. We have successfully synthesized single crystals of MnRhP, a magnetic material with a distorted kagome lattice, and systematically investigated its magnetic structure and electrical transport properties. We found that this material hosts magnetic skyrmions above room temperature and exhibits a large anomalous Hall effect. Furthermore, first-principles calculations reveal that this anomalous Hall effect originates from the Berry curvature associated with topological nodal lines. This study demonstrates that MnRhP is a rare kagome lattice magnet that possesses topological properties in both real space and momentum space.

(a) Schematic crystal structure of MnRhP. (b) Schematic spin texture of a magnetic skyrmion. (c) Temperature dependence of the anomalous Hall conductivity (AHC) in MnRhP.
Development of new room-temperature antiskyrmion materials and observation of magnetic domain structures
Skyrmions are vortex-like topological spin textures and anticipated to be used for spintronics devices. Antiskyrmions are anti-vortex topological spin textures with topological numbers of opposite sign to those of skyrmions. While antiskyrmions have been expected to form in magnets with D2d or S4 symmetry, they have only been observed in Heusler alloys with D2d symmetry. We discovered a new material (Fe,Ni,Pd)3P as a host of antiskyrmions above room temperature. Furthermore, we revealed anisotropic fractal magnetic domain structures in bulk crystals using magnetic force microscopy and small-angle neutron scattering.

(a) Schematic spin texture of an antiskyrmion. (b) Single crystal of (Fe,Ni,Pd)3P. (c) Magnetic force microscopy image of fractal magnetic domain texture. (d) Magnetic small-angle neutron scattering pattern.
Reproduced from [Karube et al. (2022). J. Appl. Cryst. 55, 1392-1400] with permission of the International Union of Crystallography